The south and southwest coast is where you want to be, especially Costa Adeje, Puerto Colón, Los Cristianos, and Los Gigantes. That’s where the proper boat trips leave from, and that’s where your chances are best.
If you want the honest version, go early and keep your expectations sensible.
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You’re not chasing a guaranteed show, just a much better shot at seeing wild dolphins in a place where they’re genuinely around.